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Than the TePP and you will pentaphenylpyrrole (PPP), both TPM and you may TPM-Cl shown prolonged emission wavelengths. Because of the equivalent toxins structures, this is not possible to help you attribute the important Stokes change so you can variations in the energy gap between the low singlet delighted county (S1) and you may ground state (S0). I therefore propose that the brand new red emission represents a low triplet thrilled condition (T1), that’s lower than S1. 2, where the curves are exactly the same on the constant-county emission spectra, sharing the new long existence services out of each other TPM and you can TPM-Cl. The brand new lifetimes of your TPM and you may TPM-Cl crystalline powders is 20.1 and you may 8.9 μs, correspondingly (Fig. S3 and Dining table S1).
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Chongqing Wulong Karst Region, Wulong Karst Land
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